Henry, if it was green it was Slime, which does indeed fill little 'oles from the inside pretty well, but also totally covers the inside of tyres and wheels with green sticky muck that is really hard to remove. All the bike shops here have signs up saying how much they charge for fixing tyres full of Slime, usually $50-$70 extra just to clean the disgusting stuff off.
Goop, on the other hand, is crystal clear. It works very well for repairing running shoe soles, some formulations of it have very high internal cohesion and make excellent contact cement substitutes (that don't require both surfaces to be tacky and brought together in perfect alignment, considerable setup movement is possible). But even straight from the tube it is VERY viscous, like stiff pitch, and I don't even know how you'd get it into a tyre. Also it air dries so you'd get a big lump of heavy Goop hardening at the lowest point of a tyre parked overnight... :-[
Unless Goop has come out with a different formulation for tyres, I suspect it would be an absolute disaster in motorbike tyres.
Ken